This book describes a relatively new approach for the design of electromagnetic metamaterials. Numerical optimization routines are combined with electromagnetic simulations to tailor the broadband optical properties of a metamaterial to have predetermined responses at predetermined wavelengths.After a review of both the major efforts within the field of metamaterials and the field of mathematical optimization, chapters covering both gradient-based and derivative-free design methods are considered. Selected topics including surrogate-base optimization, adaptive mesh search, and genetic algorithms are shown to be effective, gradient-free optimization strategies. Additionally, new techniques for representing dielectric distributions in two dimensions, including level sets, are demonstrated as effective methods for gradient-based optimization. Each chapter begins with a rigorous review of the optimization strategy used, and is followed by numerous examples that combine the strategy with either electromagnetic simulations or analytical solutions of the scattering problem. Throughout the text, we address the strengths and limitations of each method, as well as which numerical methods are best suited for different types of metamaterial designs. This book is intended to provide a detailed enough treatment of the mathematical methods used, along with sufficient examples and additional references, that senior level undergraduates or graduate students who are new to the fields of plasmonics, metamaterials, or optimization methods; have an understanding of which approaches are best-suited for their work and how to implement the methods themselves.